Ecology and Environment ›› 2022, Vol. 31 ›› Issue (12): 2358-2366.DOI: 10.16258/j.cnki.1674-5906.2022.12.010
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JIANG Bin1,3(), CHEN Duohong2,*(
), ZHANG Tao2, YUAN Luan2, ZHOU Yan2, SHEN Jing2, ZHANG Chunlin1, WANG Boguang1,3
Received:
2022-08-18
Online:
2022-12-18
Published:
2023-02-15
Contact:
CHEN Duohong
蒋斌1,3(), 陈多宏2,*(
), 张涛2, 袁鸾2, 周炎2, 沈劲2, 张春林1, 王伯光1,3
通讯作者:
陈多宏
作者简介:
蒋斌(1990年生),男,硕士,主要研究方向为大气环境化学与气候变迁。E-mail: jndxjiangbin@126.com
基金资助:
CLC Number:
JIANG Bin, CHEN Duohong, ZHANG Tao, YUAN Luan, ZHOU Yan, SHEN Jing, ZHANG Chunlin, WANG Boguang. Characteristics and Sources of Carbonaceous Aerosols during the Crop Straw Burning Seasons in Southern China[J]. Ecology and Environment, 2022, 31(12): 2358-2366.
蒋斌, 陈多宏, 张涛, 袁鸾, 周炎, 沈劲, 张春林, 王伯光. 华南水稻秸秆焚烧期碳质气溶胶组分特征及源贡献评估[J]. 生态环境学报, 2022, 31(12): 2358-2366.
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URL: https://www.jeesci.com/EN/10.16258/j.cnki.1674-5906.2022.12.010
参数项 Parameters | 夏收期 Summer harvest season | 秋收期 Autumn harvest season |
---|---|---|
温度 t/℃ | 30.0±3.3 | 24.9±2.8 |
相对湿度 Relative Humidity/% | 69.3±13.7 | 67.8±13.0 |
风速 v(wind)/(m∙s−1) | 1.8±1.1 | 1.1±0.6 |
ρ(CO)/(mg∙m−3) | 0.7± 0.1 | 1.1±0.3 |
ρ(NO2)/(μg∙m−3) | 11.9±7.3 | 38.4±22.0 |
ρ(SO2)/(μg∙m−3) | 11.5±7.3 | 31.3±19.4 |
ρ(O3)/(μg∙m−3) | 74.0±59.6 | 73.6±66.5 |
ρ(PM2.5)/(μg∙m−3) | 33.1±10.6 | 71.2±39.0 |
ρ(EC)/(μg∙m−3) | 2.5±1.3 | 5.8±3.9 |
ρ(OC)/(μg∙m−3) | 6.6±2.5 | 13.6±8.5 |
ρ(OC)/ρ(EC) | 3.0±1.7 | 2.5±0.8 |
ρ(TC)/ρ(PM2.5) | 30.9%±3.7% | 26.8%±7.1% |
ρ(K+)/ρ(PM2.5) | 1.2%±0.7% | 4.1%±2.2% |
Table 1 Meteorological parameters and pollutants during the sampling periods
参数项 Parameters | 夏收期 Summer harvest season | 秋收期 Autumn harvest season |
---|---|---|
温度 t/℃ | 30.0±3.3 | 24.9±2.8 |
相对湿度 Relative Humidity/% | 69.3±13.7 | 67.8±13.0 |
风速 v(wind)/(m∙s−1) | 1.8±1.1 | 1.1±0.6 |
ρ(CO)/(mg∙m−3) | 0.7± 0.1 | 1.1±0.3 |
ρ(NO2)/(μg∙m−3) | 11.9±7.3 | 38.4±22.0 |
ρ(SO2)/(μg∙m−3) | 11.5±7.3 | 31.3±19.4 |
ρ(O3)/(μg∙m−3) | 74.0±59.6 | 73.6±66.5 |
ρ(PM2.5)/(μg∙m−3) | 33.1±10.6 | 71.2±39.0 |
ρ(EC)/(μg∙m−3) | 2.5±1.3 | 5.8±3.9 |
ρ(OC)/(μg∙m−3) | 6.6±2.5 | 13.6±8.5 |
ρ(OC)/ρ(EC) | 3.0±1.7 | 2.5±0.8 |
ρ(TC)/ρ(PM2.5) | 30.9%±3.7% | 26.8%±7.1% |
ρ(K+)/ρ(PM2.5) | 1.2%±0.7% | 4.1%±2.2% |
采样点 Locations | 采样时间 Periods | ρ(OC)(by C)/(μg∙m−3) | ρ(OC)(by C)/(μg∙m−3) | ρ(TC)/ρ(PM2.5) | 参考文献 References |
---|---|---|---|---|---|
鹤山 Heshan | 2010年11月 | 31.85 | 6.67 | 41.6% | 丁晴等, |
鹤山 Heshan | 2014年7月 | 6.6 | 2.6 | 30.9% | This research |
2014年10月 | 13.4 | 5.8 | 26.8% | ||
广州 Guangzhou | 2012全年 | 7.3 | 2.7 | 20.8% | Wu et al., |
厦门 Xiamen | 2014年12月 | 9.8 | 1.9 | 15.6% | 胡起超等, |
成都 Chengdu | 2015年7月 | 7.4 | 2.5 | 21.9% | Wang et al., |
2014年10—11月 | 10.4 | 3.0 | 21.6% | ||
重庆 Chongqing | 2015年7月 | 9.7 | 3.8 | 24.0% | Wang et al., |
2014年10—11月 | 8.5 | 3.7 | 22.5% | ||
上海 Shanghai | 2012年夏季 | 6.2 | 1.4 | 14.7% | Zhao et al., |
2012年秋季 | 12.8 | 2.4 | 18.5% | ||
南京 Nanjing | 2013年夏季 | 15.8 | 7.1 | 29.4% | Li et al., |
2013年秋季 | 46.0 | 14.2 | 22.7% | ||
新乡 Xinxiang | 2013年10—11月 | 29.3 | 4.8 | 14.0% | 申铠君等, |
石家庄 Shijiazhuang | 2013年10月 | 23.5 | 7.3 | 16.6% | 常青, |
西安 Xi’an | 2012年夏季 | 18.9 | 8.0 | 28.4% | 王帆等, |
2012年秋季 | 29.8 | 8.4 | 30.0% | ||
北京 Beijing | 2014年7—8月 | 9.3 | 3.1 | 20.0% | Gao et al., |
名古屋, 日本 Nagoya, Japan | 2018全年 | 3.3 | 0.7 | 32.5% | Makiko et al., |
洛杉矶, 美国 Los Angeles, America | 2010全年 | 5.8 | 1.7 | 33.8% | Abdulmlik et al., |
塞萨洛尼基, 希腊 Thessaloniki, Greece | 2011全年 | 8.4 | 5.3 | 44.0% | Constantimi et al., |
波尔图, 葡萄牙 Oporto, Portugal | 2013年夏季 | 7.1 | 4.7 | 33.5% | Danilo et al., |
Table 2 ρ(EC) and ρ(OC) in PM2.5 at home and abroad
采样点 Locations | 采样时间 Periods | ρ(OC)(by C)/(μg∙m−3) | ρ(OC)(by C)/(μg∙m−3) | ρ(TC)/ρ(PM2.5) | 参考文献 References |
---|---|---|---|---|---|
鹤山 Heshan | 2010年11月 | 31.85 | 6.67 | 41.6% | 丁晴等, |
鹤山 Heshan | 2014年7月 | 6.6 | 2.6 | 30.9% | This research |
2014年10月 | 13.4 | 5.8 | 26.8% | ||
广州 Guangzhou | 2012全年 | 7.3 | 2.7 | 20.8% | Wu et al., |
厦门 Xiamen | 2014年12月 | 9.8 | 1.9 | 15.6% | 胡起超等, |
成都 Chengdu | 2015年7月 | 7.4 | 2.5 | 21.9% | Wang et al., |
2014年10—11月 | 10.4 | 3.0 | 21.6% | ||
重庆 Chongqing | 2015年7月 | 9.7 | 3.8 | 24.0% | Wang et al., |
2014年10—11月 | 8.5 | 3.7 | 22.5% | ||
上海 Shanghai | 2012年夏季 | 6.2 | 1.4 | 14.7% | Zhao et al., |
2012年秋季 | 12.8 | 2.4 | 18.5% | ||
南京 Nanjing | 2013年夏季 | 15.8 | 7.1 | 29.4% | Li et al., |
2013年秋季 | 46.0 | 14.2 | 22.7% | ||
新乡 Xinxiang | 2013年10—11月 | 29.3 | 4.8 | 14.0% | 申铠君等, |
石家庄 Shijiazhuang | 2013年10月 | 23.5 | 7.3 | 16.6% | 常青, |
西安 Xi’an | 2012年夏季 | 18.9 | 8.0 | 28.4% | 王帆等, |
2012年秋季 | 29.8 | 8.4 | 30.0% | ||
北京 Beijing | 2014年7—8月 | 9.3 | 3.1 | 20.0% | Gao et al., |
名古屋, 日本 Nagoya, Japan | 2018全年 | 3.3 | 0.7 | 32.5% | Makiko et al., |
洛杉矶, 美国 Los Angeles, America | 2010全年 | 5.8 | 1.7 | 33.8% | Abdulmlik et al., |
塞萨洛尼基, 希腊 Thessaloniki, Greece | 2011全年 | 8.4 | 5.3 | 44.0% | Constantimi et al., |
波尔图, 葡萄牙 Oporto, Portugal | 2013年夏季 | 7.1 | 4.7 | 33.5% | Danilo et al., |
采样点 Locations | 采样时间 Periods | 生物质燃烧对 有机碳的贡献 ρ(OCbb)/ρ(OC) | 生物质燃烧对 元素碳的贡献 ρ(ECbb)/ρ(EC) | 参考文献 Reference |
---|---|---|---|---|
鹤山 Heshan | 2014年7月, 水稻收割期 | 12.4% | 12.1% | This research |
成都 Chengdu | 2012年5月—2013年7月 | 30.8% | — | Chen et al., |
北京 Beijing | 2013全年 | 18.4% | — | Ji et al., |
虞城 Yucheng | 2013年6月, 生物质燃烧事件 | 44.5% | 50.8% | Yao et al., |
上海 Shanghai | 2011年5月—6月, 农作物收割期 | 69% | 68% | Cheng et al., |
南京 Nanjing | 2014年6月, 农作物收割期 | 51% | 16% | Chen et al., |
鹤山 Heshan | 2014年10月, 水稻收割期 | 66.6% | 39.5% | This research |
广州 Guangzhou | 2013年冬季, 霾污染事件 | 58% | 32% | Zhang et al., |
大田市, 韩国 Daejeon, Korea | 2012年10月—11月, 水稻收割期 | 45.0% | 12.0% | Jung et al., |
布达佩斯, 匈牙利 Budapest, Hungary | 2017年10月 | 36.0% | 43.0% | Salma et al., |
Table 3 Comparison of biomass burning contribution to carbon components
采样点 Locations | 采样时间 Periods | 生物质燃烧对 有机碳的贡献 ρ(OCbb)/ρ(OC) | 生物质燃烧对 元素碳的贡献 ρ(ECbb)/ρ(EC) | 参考文献 Reference |
---|---|---|---|---|
鹤山 Heshan | 2014年7月, 水稻收割期 | 12.4% | 12.1% | This research |
成都 Chengdu | 2012年5月—2013年7月 | 30.8% | — | Chen et al., |
北京 Beijing | 2013全年 | 18.4% | — | Ji et al., |
虞城 Yucheng | 2013年6月, 生物质燃烧事件 | 44.5% | 50.8% | Yao et al., |
上海 Shanghai | 2011年5月—6月, 农作物收割期 | 69% | 68% | Cheng et al., |
南京 Nanjing | 2014年6月, 农作物收割期 | 51% | 16% | Chen et al., |
鹤山 Heshan | 2014年10月, 水稻收割期 | 66.6% | 39.5% | This research |
广州 Guangzhou | 2013年冬季, 霾污染事件 | 58% | 32% | Zhang et al., |
大田市, 韩国 Daejeon, Korea | 2012年10月—11月, 水稻收割期 | 45.0% | 12.0% | Jung et al., |
布达佩斯, 匈牙利 Budapest, Hungary | 2017年10月 | 36.0% | 43.0% | Salma et al., |
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