Ecology and Environment ›› 2024, Vol. 33 ›› Issue (2): 249-260.DOI: 10.16258/j.cnki.1674-5906.2024.02.009
• Research Article [Environmental Sciences] • Previous Articles Next Articles
LIANG Beizhu1(), CHEN Jianyao1,*, YANG Zaizhi1, ZHANG Pengcheng1, REN Kun1, LIANG Zuobing1, YANG Chenchen1, WU Jieshan2
Received:
2023-08-31
Online:
2024-02-18
Published:
2024-04-03
梁贝竹1(), 陈建耀1,*, 杨再智1, 张鹏程1, 任坤1, 梁作兵1, 杨晨晨1, 吴洁珊2
通讯作者:
陈建耀。
作者简介:
梁贝竹(2001年生),女,硕士研究生,研究方向为流域水环境。E-mail: liangbzh3@mail2.sysu.edu.cn
基金资助:
CLC Number:
LIANG Beizhu, CHEN Jianyao, YANG Zaizhi, ZHANG Pengcheng, REN Kun, LIANG Zuobing, YANG Chenchen, WU Jieshan. Spatial Pattern and Sources of PPCPs in Groundwater and Relevant Influencing Factors in a Coastal Watershed in South China: A Case Study in Tangjiawan Town of Zhuhai, Guangdong Province[J]. Ecology and Environment, 2024, 33(2): 249-260.
梁贝竹, 陈建耀, 杨再智, 张鹏程, 任坤, 梁作兵, 杨晨晨, 吴洁珊. 华南滨海小流域地下水中PPCPs的分布、来源及影响因素——以珠海市唐家湾镇为例[J]. 生态环境学报, 2024, 33(2): 249-260.
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URL: https://www.jeesci.com/EN/10.16258/j.cnki.1674-5906.2024.02.009
采样井 | 纬度 | 经度 |
---|---|---|
TJ01 | 22.3644°N | 113.5877°E |
TJ02 | 22.3638°N | 113.5878°E |
TJ03 | 22.3636°N | 113.5881°E |
TJ04 | 22.3636°N | 113.5889°E |
TJ05 | 22.3636°N | 113.5883°E |
TJ06 | 22.3636°N | 113.5898°E |
TJ07 | 22.3631°N | 113.5897°E |
TJ08 | 22.3626°N | 113.5889°E |
TJ09 | 22.3622°N | 113.5883°E |
TJ10 | 22.3625°N | 113.5878°E |
TJ11 | 22.3628°N | 113.5881°E |
TJ12 | 22.3622°N | 113.5897°E |
TJ13 | 22.3625°N | 113.5906°E |
TJ14 | 22.3628°N | 113.5903°E |
TJ15 | 22.3631°N | 113.5922°E |
TJSQS | 22.3608°N | 113.5818°E |
Table 1 Characteristics of sampling wells in Tangjiawan Town, Zhuhai City
采样井 | 纬度 | 经度 |
---|---|---|
TJ01 | 22.3644°N | 113.5877°E |
TJ02 | 22.3638°N | 113.5878°E |
TJ03 | 22.3636°N | 113.5881°E |
TJ04 | 22.3636°N | 113.5889°E |
TJ05 | 22.3636°N | 113.5883°E |
TJ06 | 22.3636°N | 113.5898°E |
TJ07 | 22.3631°N | 113.5897°E |
TJ08 | 22.3626°N | 113.5889°E |
TJ09 | 22.3622°N | 113.5883°E |
TJ10 | 22.3625°N | 113.5878°E |
TJ11 | 22.3628°N | 113.5881°E |
TJ12 | 22.3622°N | 113.5897°E |
TJ13 | 22.3625°N | 113.5906°E |
TJ14 | 22.3628°N | 113.5903°E |
TJ15 | 22.3631°N | 113.5922°E |
TJSQS | 22.3608°N | 113.5818°E |
统计指标 | 电导率/ (μS∙cm−1) | 溶解性总固体/ (mg∙L−1) | 盐度/ (mg∙L−1) | 溶解氧/ (mg∙L−1) | pH |
---|---|---|---|---|---|
最小值 | 54.1 | 40.1 | 23.8 | 0.850 | 5.79 |
最大值 | 600 | 462 | 272 | 7.04 | 8.43 |
平均值 | 386 | 291 | 174 | 3.29 | 7.01 |
标准差 | 154 | 126 | 70.6 | 1.96 | 0.710 |
变异系数/% | 40.0 | 43.4 | 40.5 | 59.5 | 10.1 |
Table 2 Statistical characteristic of physicochemical parameters of groundwater in Tangjiawan Town, Zhuhai City
统计指标 | 电导率/ (μS∙cm−1) | 溶解性总固体/ (mg∙L−1) | 盐度/ (mg∙L−1) | 溶解氧/ (mg∙L−1) | pH |
---|---|---|---|---|---|
最小值 | 54.1 | 40.1 | 23.8 | 0.850 | 5.79 |
最大值 | 600 | 462 | 272 | 7.04 | 8.43 |
平均值 | 386 | 291 | 174 | 3.29 | 7.01 |
标准差 | 154 | 126 | 70.6 | 1.96 | 0.710 |
变异系数/% | 40.0 | 43.4 | 40.5 | 59.5 | 10.1 |
统计指标 | ρ(K+) | ρ(Na+) | ρ(Ca2+) | ρ(Mg2+) | ρ(Cl−) | ρ(SO42−) | ρ(HCO3−) |
---|---|---|---|---|---|---|---|
最小值/ (mg∙L−1) | 3.93 | 7.27 | 1.26 | 0.520 | 5.65 | 1.06 | 30.5 |
最大值/ (mg∙L−1) | 64.8 | 51.3 | 96.4 | 7.27 | 87.7 | 69.7 | 317 |
平均值/ (mg∙L−1) | 36.4 | 31.6 | 55.9 | 4.69 | 42.1 | 41.2 | 157 |
标准差/ (mg∙L−1) | 17.3 | 13.4 | 27.3 | 1.96 | 20.7 | 19.7 | 84.3 |
变异系数/% | 47.6 | 42.6 | 48.9 | 41.8 | 49.2 | 47.7 | 53.8 |
Table 3 Statistical characteristic of ionic concentration in groundwater in Tangjiawan Town, Zhuhai City
统计指标 | ρ(K+) | ρ(Na+) | ρ(Ca2+) | ρ(Mg2+) | ρ(Cl−) | ρ(SO42−) | ρ(HCO3−) |
---|---|---|---|---|---|---|---|
最小值/ (mg∙L−1) | 3.93 | 7.27 | 1.26 | 0.520 | 5.65 | 1.06 | 30.5 |
最大值/ (mg∙L−1) | 64.8 | 51.3 | 96.4 | 7.27 | 87.7 | 69.7 | 317 |
平均值/ (mg∙L−1) | 36.4 | 31.6 | 55.9 | 4.69 | 42.1 | 41.2 | 157 |
标准差/ (mg∙L−1) | 17.3 | 13.4 | 27.3 | 1.96 | 20.7 | 19.7 | 84.3 |
变异系数/% | 47.6 | 42.6 | 48.9 | 41.8 | 49.2 | 47.7 | 53.8 |
PPCPs种类 | 质量浓度范围/ (ng∙L−1) | 中间值/ (ng∙L−1) | 均值/ (ng∙L−1) | 检出率/ % |
---|---|---|---|---|
Sulfadimethoxine 磺胺间二甲氧嘧啶 | ND | 0 | 0 | 0 |
Sulfamethoxazole 磺胺甲恶唑 | ND‒58.6 | 29.3 | 5.51 | 81.0 |
Sulfamonomethoxine 磺胺间甲氧嘧啶 | ND | 0 | 0 | 0 |
Sulfamerazine 磺胺甲基嘧啶 | 0.919‒1.60 | 1.26 | 1.18 | 100 |
Sulfamethazine 磺胺二甲基嘧啶 | ND‒0.883 | 0.442 | 0.168 | 25.0 |
Sulfachinoxalin 磺胺喹恶啉 | ND | 0 | 0 | 0 |
Tracycline 四环素 | ND | 0 | 0 | 0 |
Oxytetracycline 土霉素 | ND | 0 | 0 | 0 |
Chlorotetracycline 金霉素 | ND | 0 | 0 | 0 |
Doxycycline 强力霉素 | ND | 0 | 0 | 0 |
Enrofloxacin 恩诺沙星 | ND | 0 | 0 | 0 |
Ciprofloxacin 环丙沙星 | ND | 0 | 0 | 0 |
Clenbuterol 克伦特罗 | ND | 0 | 0 | 0 |
Salbutamol 沙丁氨醇 | ND | 0 | 0 | 0 |
Cimaterol 西马特罗 | ND‒1.54 | 0.770 | 0.100 | 6.25 |
Ractopamine 莱克多巴胺 | ND | 0 | 0 | 0 |
Carbamazepine 卡马西平 | ND‒334 | 167 | 35.7 | 93.8 |
Caffeine 咖啡因 | 6.49‒214 | 110 | 110 | 100 |
Atrazine 阿特拉津 | ND | 0 | 0 | 0 |
Chloramphenicol 氯霉素 | ND | 0 | 0 | 0 |
Florfenicol 氟苯尼考 | ND | 0 | 0 | 0 |
Table 4 Detection condition of PPCPs in groundwater in Tangjiawan Town, Zhuhai City
PPCPs种类 | 质量浓度范围/ (ng∙L−1) | 中间值/ (ng∙L−1) | 均值/ (ng∙L−1) | 检出率/ % |
---|---|---|---|---|
Sulfadimethoxine 磺胺间二甲氧嘧啶 | ND | 0 | 0 | 0 |
Sulfamethoxazole 磺胺甲恶唑 | ND‒58.6 | 29.3 | 5.51 | 81.0 |
Sulfamonomethoxine 磺胺间甲氧嘧啶 | ND | 0 | 0 | 0 |
Sulfamerazine 磺胺甲基嘧啶 | 0.919‒1.60 | 1.26 | 1.18 | 100 |
Sulfamethazine 磺胺二甲基嘧啶 | ND‒0.883 | 0.442 | 0.168 | 25.0 |
Sulfachinoxalin 磺胺喹恶啉 | ND | 0 | 0 | 0 |
Tracycline 四环素 | ND | 0 | 0 | 0 |
Oxytetracycline 土霉素 | ND | 0 | 0 | 0 |
Chlorotetracycline 金霉素 | ND | 0 | 0 | 0 |
Doxycycline 强力霉素 | ND | 0 | 0 | 0 |
Enrofloxacin 恩诺沙星 | ND | 0 | 0 | 0 |
Ciprofloxacin 环丙沙星 | ND | 0 | 0 | 0 |
Clenbuterol 克伦特罗 | ND | 0 | 0 | 0 |
Salbutamol 沙丁氨醇 | ND | 0 | 0 | 0 |
Cimaterol 西马特罗 | ND‒1.54 | 0.770 | 0.100 | 6.25 |
Ractopamine 莱克多巴胺 | ND | 0 | 0 | 0 |
Carbamazepine 卡马西平 | ND‒334 | 167 | 35.7 | 93.8 |
Caffeine 咖啡因 | 6.49‒214 | 110 | 110 | 100 |
Atrazine 阿特拉津 | ND | 0 | 0 | 0 |
Chloramphenicol 氯霉素 | ND | 0 | 0 | 0 |
Florfenicol 氟苯尼考 | ND | 0 | 0 | 0 |
PPCPs | Pearson相关性 | P值 (双侧显著性) |
---|---|---|
磺胺甲恶唑 | −0.140 | 0.518 |
磺胺甲基嘧啶 | 0.452 | 0.083 |
磺胺二甲基嘧啶 | 0.394 | 0.878 |
西马特罗 | −0.165 | ‒ |
卡马西平 | 0.839 | 0.000* |
咖啡因 | 0.540 | 0.061 |
Table 5 The relationship between total PPCPs and individual PPCPs of groundwater in Tangjiawan Town, Zhuhai City
PPCPs | Pearson相关性 | P值 (双侧显著性) |
---|---|---|
磺胺甲恶唑 | −0.140 | 0.518 |
磺胺甲基嘧啶 | 0.452 | 0.083 |
磺胺二甲基嘧啶 | 0.394 | 0.878 |
西马特罗 | −0.165 | ‒ |
卡马西平 | 0.839 | 0.000* |
咖啡因 | 0.540 | 0.061 |
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